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 <\/p>\n

\u66f4\u5173\u952e\u7684\u662f\uff0c\u4e0eIrO2<\/sub>\u4e0d\u540c\uff0cRuO2<\/sub>\u4e2d\u7684\u6676\u683c\u6c27\u53ef\u4ee5\u901a\u8fc7\u6676\u683c\u6c27\u6c27\u5316\u673a\u5236(LOM)\u9014\u5f84\u53c2\u4e0eOER\uff0c\u7834\u574f\u4e86AEM\u9014\u5f84\u4e2d*OOH\u548c*O\u7684\u5438\u9644\u80fd\u4e4b\u95f4\u7684\u6807\u5ea6\u5173\u7cfb\uff0c\u663e\u8457\u589e\u5f3a\u5185\u5728OER\u52a8\u529b\u5b66\u3002\u56e0\u6b64\uff0c\u5728OER\u8fc7\u7a0b\u4e2d\u6d3b\u5316\u6676\u683c\u6c27\u548c\u964d\u4f4e\u6c27\u7a7a\u4f4d\u5f62\u6210\u80fd\u6709\u671b\u8fdb\u4e00\u6b65\u63d0\u9ad8OER\u6d3b\u6027\uff0c\u4f46\u8fd9\u5f88\u5c11\u6709\u62a5\u9053\u3002<\/section>\n
\"1\"<\/section>\n
\"2\"<\/section>\n
\u8fd1\u65e5\uff0c\u6b66\u6c49\u5927\u5b66\u7f57\u5a01<\/strong>\u8bfe\u9898\u7ec4\u5c06\u539f\u5b50Ru\u7269\u79cd\u52a0\u5165\u5230\u5177\u6709\u72ec\u7279\u4ea4\u53c9\u03c0\u5171\u8f6d\u7684\u4e59\u70ef\u57fa\u8fde\u63a5\u76842D COF\u4e2d\uff0c\u8bbe\u8ba1\u5e76\u6784\u5efa\u4e86\u4e00\u79cd\u5728\u9178\u6027\u6761\u4ef6\u4e0b\u7a33\u5b9a\u7684COF\u57fa\u7535\u50ac\u5316\u5242(COF-205-Ru)\u3002<\/section>\n
\u6839\u636e\u5b9e\u9a8c\u7ed3\u679c\uff0c\u7814\u7a76\u4eba\u5458\u53d1\u73b0\u5177\u6709\u591a\u4e2a\u03c0\u5171\u8f6d\u7684\u4ea4\u53c9\u03c0\u5171\u8f6d<\/span>\u4f53\u7cfb\u8868\u73b0\u51fa\u589e\u5f3a\u7684\u7535\u5b50\u8f68\u9053\u91cd\u53e0\uff0c\u8fd9\u662f\u4f18\u5316\u7535\u5b50\u7ed3\u6784\u548c\u63d0\u9ad8\u7535\u5b50\u8f6c\u79fb\u6548\u7387\u7684\u539f\u56e0\uff1b\u540c\u65f6\uff0cCOF-205-Ru\u7684\u7cbe\u786e\u7ed3\u6784\u4e0d\u4ec5\u901a\u8fc7\u5f3a\u7684Ru-N\u952e\u6291\u5236\u4e86Ru\u7684\u6eb6\u89e3\uff0c\u800c\u4e14\u901a\u8fc7\u4ea4\u53c9\u03c0\u5171\u8f6d\u964d\u4f4e\u4e86Ru\u7684\u6c27\u5316\u72b6\u6001\uff0c\u4ece\u800c\u5bfc\u81f4\u4e86\u7531\u914d\u4f4d\u6c27\u504f\u79bb\u4ea7\u751f\u7684\u7a33\u5b9a\u6c27\u7a7a\u4f4d\u3002<\/section>\n
\"3\"<\/section>\n
\"6\"<\/section>\n
\u7279\u522b\u5730\uff0c\u6240\u83b7\u5f97\u7684COF-205-Ru\u50ac\u5316\u5242\u663e\u793a\u51fa\u9ad8\u8d28\u91cf\u6d3b\u6027(2659.3 A g-1<\/sup>)\u548c\u5bf9\u9178\u6027OER\u7684\u957f\u671f\u8010\u4e45\u6027(\u8d85\u8fc7280\u5c0f\u65f6)\u3002XAS\u3001\u539f\u4f4d\u62c9\u66fc\u5149\u8c31\u5b66\u548c\u539f\u4f4d\u7c89\u672bXRD\u7684\u5b9e\u9a8c\u7ed3\u679c\u63ed\u793a\u4e86\u914d\u4f4d\u6c27\u5728\u9ad8\u7a33\u5b9a\u6027\u7684OER\u8fc7\u7a0b\u4e2d\u7684\u6d3b\u5316\u548c\u53c2\u4e0e\u3002\u6b64\u5916\uff0c\u7406\u8bba\u8ba1\u7b97\u8868\u660e\uff0cCOF-205-Ru\u72ec\u7279\u7684\u4ea4\u53c9\u5171\u8f6d\u4e0d\u4ec5\u80fd\u63d0\u4f9b\u5f3a\u7535\u5b50\u79bb\u57df\uff0c\u7a33\u5b9a\u6c27\u7a7a\u4f4d\uff0c\u964d\u4f4e\u901f\u7387\u63a7\u5236\u6b65\u9aa4\u7684\u80fd\u5792\uff0c\u800c\u4e14\u901a\u8fc7\u7a33\u5065\u7684\u03c0\u5171\u8f6d\u6846\u67b6\u548cRu-N\u914d\u4f4d\u4fdd\u6301\u7ed3\u6784\u7a33\u5b9a\u3002<\/section>\n
\u603b\u7684\u6765\u8bf4\uff0c\u8be5\u9879\u5de5\u4f5c\u9996\u6b21\u62a5\u9053\u4e86COFs\u5e94\u7528\u4e8e\u9178\u6027OER\uff0c\u5e76\u63a2\u7d22\u6d3b\u6027\u4e2d\u5fc3\u7ed3\u6784\u4e0e\u5176\u50ac\u5316\u6d3b\u6027\/\u7a33\u5b9a\u6027\u4e4b\u95f4\u7684\u7ed3\u6784-\u6027\u8d28\u5173\u7cfb\uff0c\u4e3aCOF\u57fa\u9178\u6027OER\u50ac\u5316\u5242\u7684\u7cbe\u786e\u8bbe\u8ba1\u548c\u6839\u636e\u50ac\u5316\u5242\u7ed3\u6784\u57fa\u672c\u786e\u5b9a\u6d3b\u6027\u4e2d\u5fc3\u63d0\u4f9b\u7814\u7a76\u8303\u5f0f\u3002<\/section>\n
Stabilizing atomic Ru species in conjugated sp2<\/sup>\u00a0carbon-linked covalent organic framework for acidic water oxidation. Nature Communications, 2024. DOI: 10.1038\/s41467-024-49834-5<\/section>\n

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