{"id":48428,"date":"2023-07-15T08:15:27","date_gmt":"2023-07-15T00:15:27","guid":{"rendered":"https:\/\/www.chemhui.com\/?p=48428"},"modified":"2023-06-28T10:16:13","modified_gmt":"2023-06-28T02:16:13","slug":"%e9%9d%92%e7%a7%91%e5%a4%a7chem-eng-j-%ef%bc%9a%e8%b0%83%e8%8a%82rucomoyox%e7%9a%84%e9%9d%9e%e6%99%b6-%e6%99%b6%e6%80%81%e9%9d%9e%e5%9d%87%e7%9b%b8%e7%95%8c%e9%9d%a2%e5%ae%9e%e7%8e%b0%e9%ab%98","status":"publish","type":"post","link":"http:\/\/www.chemhui.com\/%e9%9d%92%e7%a7%91%e5%a4%a7chem-eng-j-%ef%bc%9a%e8%b0%83%e8%8a%82rucomoyox%e7%9a%84%e9%9d%9e%e6%99%b6-%e6%99%b6%e6%80%81%e9%9d%9e%e5%9d%87%e7%9b%b8%e7%95%8c%e9%9d%a2%e5%ae%9e%e7%8e%b0%e9%ab%98\/","title":{"rendered":"\u9752\u79d1\u5927Chem. Eng. J.\uff1a\u8c03\u8282RuCoMoyOx\u7684\u975e\u6676\/\u6676\u6001\u975e\u5747\u76f8\u754c\u9762\u5b9e\u73b0\u9ad8\u6548\u5168\u6c34\u89e3"},"content":{"rendered":"
\u4e3a\u4e86\u5b9e\u73b0\u201c\u78b3\u4e2d\u548c\u201d\u7684\u76ee\u6807\uff0c\u5f00\u53d1\u548c\u5229\u7528\u6e05\u6d01\u80fd\u6e90\u5df2\u6210\u4e3a\u8fd9\u4e2a\u65f6\u4ee3\u7684\u4e3b\u65cb\u5f8b\u3002\u6c22\u6c14\u4f5c\u4e3a\u4e00\u79cd\u96f6\u78b3\u6392\u653e\u3001\u9ad8\u50a8\u80fd\u7684\u65b0\u578b\u6e05\u6d01\u80fd\u6e90\uff0c\u5728\u5de5\u4e1a\u751f\u4ea7\u4e2d\u5177\u6709\u66ff\u4ee3\u5316\u77f3\u71c3\u6599\u7684\u5de8\u5927\u6f5c\u529b\u3002\u5728\u6240\u6709\u4ea7\u6c22\u6280\u672f\u4e2d\uff0c\u7535\u89e3\u6c34\u6280\u672f\u4ee5\u5176\u96f6\u78b3\u6392\u653e\u548c\u6210\u719f\u53d1\u5c55\u800c\u8131\u9896\u800c\u51fa\u3002\u503c\u5f97\u6ce8\u610f\u7684\u662f\uff0c\u7535\u50ac\u5316\u5242\u662f\u5f71\u54cd\u7535\u89e3\u6c34\u53cd\u5e94\u6548\u7387\u7684\u4e00\u4e2a\u91cd\u8981\u56e0\u7d20\u3002\u76ee\u524d\u5de5\u4e1a\u7535\u50ac\u5316\u5242\u591a\u4e3a\u8d35\u91d1\u5c5e\u57fa\u7535\u50ac\u5316\u5242\uff0c\u5c24\u5176\u662fPt\/C\u548cRuO2<\/sub>(\u6216IrO2<\/sub>)\u3002\u7136\u800c\uff0c\u9ad8\u6602\u7684\u6210\u672c\u548c\u5c11\u91cf\u7684\u5730\u58f3\u50a8\u5b58\u9650\u5236\u4e86\u5176\u5e7f\u6cdb\u5e94\u7528\u3002\u56e0\u6b64\uff0c\u975e\u8d35\u91d1\u5c5e\u50ac\u5316\u5242\u88ab\u8ba4\u4e3a\u662f\u8d35\u91d1\u5c5e\u50ac\u5316\u5242\u7684\u826f\u597d\u66ff\u4ee3\u50ac\u5316\u5242\u3002\u867d\u7136\u975e\u8d35\u91d1\u5c5e\u57fa\u590d\u5408\u6750\u6599\u4e5f\u5177\u6709\u5feb\u901f\u7684\u52a8\u529b\u5b66\uff0c\u4f46\u4e0e\u8d35\u91d1\u5c5e\u76f8\u6bd4\u4ecd\u6709\u660e\u663e\u7684\u5dee\u8ddd\u3002\u56e0\u6b64\uff0c\u5c06\u5fae\u91cf\u7684\u8d35\u91d1\u5c5e\u63ba\u6742\u5230\u975e\u8d35\u91d1\u5c5e\u57fa\u50ac\u5316\u5242\u4e2d\u662f\u4e00\u79cd\u964d\u4f4e\u6210\u672c\u3001\u63d0\u9ad8\u50ac\u5316\u5242\u672c\u5f81\u6d3b\u6027\u7684\u5de7\u5999\u65b9\u6cd5\u3002<\/section>\n

 <\/p>\n

\u57fa\u4e8e\u6b64\uff0c\u9752\u5c9b\u79d1\u6280\u5927\u5b66\u675c\u4e91\u6885\u548c\u674e\u5f6c(\u5171\u540c\u901a\u8baf)\u7b49\u4eba<\/strong>\u91c7\u7528\u5171\u6c89\u6dc0-\u5fae\u6ce2\u6cd5\u5408\u6210\u4e86a\/c(\u975e\u6676\/\u6676\u6001)-RuCoMoy<\/sub>Ox<\/sub>\/NF(\u6ce1\u6cab\u954d)\u7535\u50ac\u5316\u5242\u3002<\/section>\n
\"1\"<\/section>\n
\u672c\u6587\u57281.0 M KOH\u6eb6\u6db2\u4e2d\uff0c\u5229\u7528\u6807\u51c6\u7684\u4e09\u7535\u6781\u4f53\u7cfb\u5bf9\u50ac\u5316\u5242\u8fdb\u884c\u4e86\u6790\u6c22\u53cd\u5e94(HER)\u548c\u6790\u6c27\u53cd\u5e94(OER)\u6027\u80fd\u6d4b\u8bd5\u3002\u672c\u6587\u9996\u5148\u6d4b\u8bd5\u5e76\u5206\u6790\u4e86\u4e0d\u540c\u50ac\u5316\u5242\u7684HER\u6027\u80fd\u3002\u6d4b\u8bd5\u7ed3\u679c\u8868\u660e\uff0ca\/c-RuCoMoy<\/sub>Ox<\/sub>\/NF\u50ac\u5316\u5242\u7684HER\u6d3b\u6027\u6700\u4f73\uff0c\u901a\u8fc739 mV\u548c128 mV\u7684\u8fc7\u7535\u4f4d\u5c31\u53ef\u4ee5\u8fbe\u523010\u548c100 mA cm-2<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\uff0c\u4f4e\u4e8ePt\/C-NF(78\u548c173 mV)\u3001a\/c-CoMoy<\/sub>Ox<\/sub>\/NF(141\u548c268 mV)\u548cCo-ZIF-L\/NF(201\u548c299 mV)\u3002\u5f53a\/c-RuCoMoy<\/sub>Ox<\/sub>\/NF\u4f5c\u4e3aOER\u9633\u6781\u50ac\u5316\u5242\u65f6\uff0c\u4ec5\u9700\u8981166 mV\u548c337 mV\u7684\u8fc7\u7535\u4f4d\u5c31\u80fd\u5206\u522b\u8fbe\u523010\u548c100 mA cm-2<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\uff0c\u8fd9\u540c\u6837\u4f4e\u4e8ea\/c-CoMoy<\/sub>Ox<\/sub>\/NF(376 mV\u548c451 mV)\u3001Co-ZIF-L\/NF(385 mV\u548c465 mV)\u548cRuO2<\/sub>-NF(448 mV\u548c554 mV)\u3002<\/section>\n
\u9274\u4e8ea\/c-RuCoMoy<\/sub>Ox<\/sub>\/NF\u4f18\u5f02\u7684\u6027\u80fd\uff0c\u672c\u6587\u7ec4\u88c5\u4e86a\/c-RuCoMoy<\/sub>Ox<\/sub>\/NF||a\/c-RuCoMoy<\/sub>Ox<\/sub>\/NF\u78b1\u6027\u7535\u89e3\u69fd\u6765\u7814\u7a76\u5176\u5168\u6c34\u89e3\u6027\u80fd\u3002\u4e0d\u51fa\u6240\u6599\uff0ca\/c-RuCoMoy<\/sub>Ox<\/sub>\/NF||a\/c-RuCoMoy<\/sub>Ox<\/sub>\/NF\u53ea\u9700\u89811.58 V\u7684\u7535\u538b\u5c31\u80fd\u8fbe\u5230100 mA cm-2<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\uff0c\u8fdc\u5c0f\u4e8ea\/c-CoMoy<\/sub>Ox<\/sub>\/NF||a\/c-CoMoy<\/sub>Ox<\/sub>\/NF(1.658 V)\u548cCo-ZIF-L\/NF||Co-ZIF-L\/NF(1.68 V)\u3002\u6b64\u5916\uff0c\u5728\u5927\u591a\u6570\u62a5\u9053\u7684\u50ac\u5316\u5242\u4e2d\uff0ca\/c-RuCoMoy<\/sub>Ox<\/sub>\/NF||a\/c-RuCoMoy<\/sub>Ox<\/sub>\/NF\u8fbe\u5230100 mA cm-2<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\u6240\u9700\u7684\u7535\u538b\u662f\u6700\u5c0f\u7684\u3002<\/section>\n
\"2\"<\/section>\n
\u4e3a\u4e86\u8fdb\u4e00\u6b65\u63a2\u7a76\u5177\u6709\u975e\u6676\/\u6676\u6001\u5f02\u8d28\u7ed3\u6784\u7684a\/c-RuCoMoy<\/sub>Ox<\/sub>\/NF\u5728HER\u548cOER\u8fc7\u7a0b\u4e2d\u50ac\u5316\u6d3b\u6027\u7684\u6765\u6e90\u548c\u53cd\u5e94\u673a\u7406\uff0c\u672c\u6587\u8fdb\u884c\u4e86\u5bc6\u5ea6\u6cdb\u51fd\u7406\u8bba(DFT)\u8ba1\u7b97\u3002\u672c\u6587\u6784\u5efa\u4e86\u6676\u6001Ru-CoMoO4<\/sub>\u6a21\u578b\u3001\u975e\u6676Ru-CoMoOx<\/sub>\u6a21\u578b\u4ee5\u53ca\u7531\u6676\u6001Ru-CoMoO4<\/sub>\u548c\u975e\u6676Ru-CoMoOx<\/sub>\u7ec4\u6210\u7684Ru-CoMoO4<\/sub>\/Ru-CoMoOx<\/sub>\u5f02\u8d28\u7ed3\u6784\u6a21\u578b\u3002<\/section>\n
\u8ba1\u7b97\u7ed3\u679c\u8868\u660e\uff0cRu-CoMoO4<\/sub>\u6a21\u578b\u5728\u8d39\u7c73\u80fd\u7ea7\u4e0a\u6ca1\u6709\u5cf0\uff0c\u8fd9\u8bf4\u660e\u5176\u534a\u5bfc\u4f53\u6027\u8d28\u548c\u8f83\u5dee\u7684\u7535\u5bfc\u7387\u3002\u4e0eRu-CoMoO4<\/sub>\u6a21\u578b\u4e0d\u540c\uff0cRu-CoMoOx<\/sub>\u6a21\u578b\u5728\u8d39\u7c73\u80fd\u7ea7\u4e0a\u5177\u6709\u4e00\u5b9a\u7684\u7535\u5b50\u6001\u5bc6\u5ea6\uff0c\u8fd9\u8868\u660e\u539f\u5b50\u5206\u5e03\u65e0\u5e8f\u7684Ru-CoMoOx<\/sub>\u6a21\u578b\u5177\u6709\u4e00\u5b9a\u7684\u7535\u5bfc\u7387\u3002\u503c\u5f97\u6ce8\u610f\u7684\u662f\uff0cRu-CoMoO4<\/sub>\/Ru-CoMoOx<\/sub>\u6a21\u578b\u5728\u8d39\u7c73\u80fd\u7ea7\u4e0a\u8868\u73b0\u51fa\u6bd4Ru-CoMoOx<\/sub>\u6a21\u578b\u66f4\u9ad8\u7684\u6001\u5bc6\u5ea6\uff0c\u8fd9\u4e00\u73b0\u8c61\u8fdb\u4e00\u6b65\u63ed\u793a\u4e86\u975e\u6676\/\u6676\u6001\u5f02\u8d28\u754c\u9762\u6709\u5229\u4e8e\u52a0\u901f\u7535\u5b50\u8f6c\u79fb\uff0c\u4f7f\u5f97\u6750\u6599\u7684\u7535\u5bfc\u7387\u6709\u6240\u63d0\u9ad8\u3002\u4e3a\u4e86\u6df1\u5165\u9610\u660ea\/c-RuCoMoy<\/sub>Ox<\/sub>\/NF\u7684HER\u548cOER\u771f\u5b9e\u6d3b\u6027\u4f4d\u70b9\uff0c\u672c\u6587\u5728Ru-CoMoO4<\/sub>\/Ru-CoMoOx<\/sub>\u6a21\u578b\u4e2d\u8ba1\u7b97\u4e86HER\u548cOER\u8fc7\u7a0b\u4e2d\u6676\u6001Ru-CoMoO4<\/sub>\u76f8\u7684Co\u4f4d\u70b9\u548cRu\u4f4d\u70b9\u4ee5\u53ca\u975e\u6676Ru-CoMoOx<\/sub>\u76f8\u7684Co\u4f4d\u70b9\u548cRu\u4f4d\u70b9\u7684\u5409\u5e03\u65af\u81ea\u7531\u80fd\u3002<\/section>\n
\u6839\u636e\u8ba1\u7b97\u7ed3\u679c\u53ef\u4ee5\u53d1\u73b0\uff0c\u975e\u6676Ru-CoMoOx<\/sub>\u76f8Ru\u4f4d\u70b9\u4e0aH\u5438\u9644\u5409\u5e03\u65af\u81ea\u7531\u80fd(\u0394GH*<\/sub>)\u4ec5\u4e3a-0.16 eV\uff0c\u8fd9\u8868\u660eRu-CoMoO4<\/sub>\/Ru-CoMoOx<\/sub>\u5f02\u8d28\u7ed3\u6784\u4e2d\u975e\u6676Ru-CoMoOx<\/sub>\u7684Ru\u539f\u5b50\u4f5c\u4e3aHER\u6d3b\u6027\u4f4d\u70b9\u52a0\u901f\u6c22\u7684\u9038\u51fa\u3002\u6b64\u5916\uff0c\u5728Ru-CoMoO4<\/sub>\/Ru-CoMoOx<\/sub>\u6a21\u578b\u4e2d\uff0cOER\u5728\u4e0d\u540c\u4f4d\u70b9\u7684\u901f\u7387\u51b3\u5b9a\u6b65\u9aa4\u662f*<\/sup>O\u2192*<\/sup>OOH\u3002\u5176\u4e2d\uff0c\u6676\u6001Ru-CoMoO4<\/sub>\u76f8\u4e2dRu\u4f4d\u70b9\u7684*<\/sup>O\u2192*<\/sup>OOH\u8fc7\u7a0b\u7684\u80fd\u5792\u6700\u4f4e(1.56 eV)\uff0c\u8fd9\u63ed\u793a\u4e86Ru-CoMoO4<\/sub>\/Ru-CoMoOx<\/sub>\u5f02\u8d28\u7ed3\u6784\u4e2d\u6676\u6001Ru-CoMoO4<\/sub>\u76f8\u4e2d\u7684Ru\u539f\u5b50\u662fOER\u7684\u6d3b\u6027\u4e2d\u5fc3\u3002\u7efc\u4e0a\u6240\u8ff0\uff0c\u672c\u7814\u7a76\u4e3a\u975e\u6676\/\u6676\u6001\u5f02\u8d28\u754c\u9762\u7684\u6784\u5efa\u548c\u754c\u9762\u533a\u57df\u7684\u63a7\u5236\u63d0\u4f9b\u4e86\u65b0\u7684\u601d\u8def\u548c\u4fbf\u6377\u7684\u65b9\u6cd5\uff0c\u5e76\u4e3a\u901a\u8fc7\u8c03\u8282\u975e\u6676\u533a\u57df\u5236\u5907\u9ad8\u6548\u7535\u50ac\u5316\u5242\u6307\u660e\u4e86\u65b9\u5411\u3002<\/section>\n
\"9\"<\/section>\n
Modulating Amorphous\/Crystalline Heterogeneous Interface in RuCoMoyOx Grown on Nickel Foam to Achieve Efficient Overall Water Splitting,\u00a0Chemical Engineering Journal<\/em><\/strong>,\u00a02023<\/strong>, DOI: 10.1016\/j.cej.2023.143993.<\/section>\n
https:\/\/doi.org\/10.1016\/j.cej.2023.143993.<\/section>\n

 <\/p>\n","protected":false},"excerpt":{"rendered":"

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