{"id":48415,"date":"2023-07-13T08:45:28","date_gmt":"2023-07-13T00:45:28","guid":{"rendered":"https:\/\/www.chemhui.com\/?p=48415"},"modified":"2023-06-26T13:48:15","modified_gmt":"2023-06-26T05:48:15","slug":"%e6%9c%b1%e6%b0%b8%e6%b3%95-%e9%83%ad%e7%87%95nature-catalysis%ef%bc%9a%e5%be%ae%e5%ad%94%e9%99%90%e5%9f%9f%e6%bf%80%e5%ad%90%e8%a1%8c%e4%b8%ba%e5%8a%a9%e5%8a%9b%e5%85%89%e5%82%ac%e5%8c%96","status":"publish","type":"post","link":"http:\/\/www.chemhui.com\/%e6%9c%b1%e6%b0%b8%e6%b3%95-%e9%83%ad%e7%87%95nature-catalysis%ef%bc%9a%e5%be%ae%e5%ad%94%e9%99%90%e5%9f%9f%e6%bf%80%e5%ad%90%e8%a1%8c%e4%b8%ba%e5%8a%a9%e5%8a%9b%e5%85%89%e5%82%ac%e5%8c%96\/","title":{"rendered":"\u200b\u6731\u6c38\u6cd5\/\u90ed\u71d5Nature Catalysis\uff1a\u5fae\u5b54\u9650\u57df\u6fc0\u5b50\u884c\u4e3a\u52a9\u529b\u5149\u50ac\u5316\u5236\u6c22\uff01"},"content":{"rendered":"<section data-role=\"title\" data-tools=\"135\u7f16\u8f91\u5668\" data-id=\"us-4152855\">\n<section>\n<section>\n<section>\n<section data-brushtype=\"text\"><strong>\u6210\u679c\u7b80\u4ecb<\/strong><\/section>\n<\/section>\n<\/section>\n<\/section>\n<\/section>\n<p>&nbsp;<\/p>\n<section>\u6709\u673a\u534a\u5bfc\u4f53\uff08organic semiconductors\uff09\u662f\u4e00\u7c7b\u5341\u5206\u5177\u6709\u5438\u5f15\u529b\u7684\u5149\u50ac\u5316\u5242\uff0c\u4f46\u662f\u5b83\u4eec\u7684\u91cf\u5b50\u4ea7\u7387\uff08quantum yield\uff09\u53d7\u5230\u5149\u751f\u7535\u8377\u8f6c\u79fb\u5230\u8868\u9762\u7684\u9650\u5236\u3002\u5176\u4e2d\uff0c\u4f4e\u635f\u8017\u7535\u8377\u8f6c\u79fb\u7b56\u7565\u53ef\u4ee5\u7f29\u77ed\u4ece\u4f53\u6fc0\u5b50\u8026\u5408\u533a\u57df\u5230\u50ac\u5316\u5242\u8868\u9762\u7684\u8ddd\u79bb\uff0c\u662f\u4e00\u79cd\u5f88\u6709\u524d\u666f\u7684\u7b56\u7565\u3002<\/section>\n<section>\u57fa\u4e8e\u6b64\uff0c<strong>\u6e05\u534e\u5927\u5b66\u6731\u6c38\u6cd5\u6559\u6388\u3001\u9999\u6e2f\u5927\u5b66\/\u6e05\u534e\u5927\u5b66\u90ed\u71d5\u6559\u6388\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09\u7b49\u4eba<\/strong>\u62a5\u9053\u4e86\u4e00\u79cd\u5177\u6709\u4eb2\u6c34\u6027\u4e00\u7ef4\uff081D\uff09\u5fae\u5b54\u901a\u9053\u7684\u6c22\u952e\u6709\u673a\u9aa8\u67b61, 3, 6, 8-\u56db(\u5bf9\u82ef\u7532\u9178)\u8298\uff08HOF-H<sub>4<\/sub>TBAPy\uff09\u4f5c\u4e3a\u8be5\u65b9\u6cd5\u7684\u6982\u5ff5\u8bc1\u660e\u3002\u4f5c\u8005\u91c7\u7528\u77ac\u6001\u5149\u8c31\u65b9\u6cd5\uff0c\u7ed3\u5408\u53ef\u89c1\u5149-\u4e2d\u7ea2\u5916\u98de\u79d2\u77ac\u6001\u5438\u6536\u5149\u8c31\uff08TAS\uff09\u548c\u65f6\u95f4\u76f8\u5173\u5355\u5149\u5b50\u8ba1\u6570\uff08TCSPC\uff09\uff0c\u7814\u7a76\u4e86\u5fae\u5b54\u9053\u5bf9\u6fc0\u5b50\u884c\u4e3a\u7684\u5f71\u54cd\uff0c\u7279\u522b\u662f1D\u5fae\u5b54\u9053\u5bf9HOF-H<sub>4<\/sub>TBAPy\u7684\u6fc0\u5b50\u8f6c\u79fb\u8def\u5f84\u7684\u5f71\u54cd\u3002<\/section>\n<section>\u6b64\u5916\uff0c\u4f5c\u8005\u5229\u7528\u6676\u4f53\u5de5\u7a0b\u8fdb\u4e00\u6b65\u7814\u7a76\u4e86\u5185\u90e8\u6d3b\u6027\u5438\u9644\u533a\u7684\u5f71\u54cd\uff0c\u7279\u522b\u662f\u901a\u8fc7\u63a7\u52361D\u901a\u9053\u7684\u957f\u5ea6\u3002\u5b9e\u9a8c\u8868\u660e\uff0c\u5fae\u5b54\u9053\u53ef\u4ee5\u9650\u5236\u6fc0\u5b50\u7684\u8d85\u5feb\u8f6c\u79fb\u5230\u5185\u8868\u9762\uff0c\u4e0e\u4f20\u7edf\u7684\u7535\u8377\u8fc1\u79fb\u5230\u6676\u4f53\u5e73\u9762\u7684\u89c2\u70b9\u4e0d\u540c\u3002\u7b2c\u4e00\u6027\u539f\u7406\u8ba1\u7b97\u548c\u8870\u51cf\u5168\u53cd\u5c04\u5085\u91cc\u53f6\u53d8\u6362\u7ea2\u5916\u5149\u8c31\uff08ATR-FTIR\uff09\u4e5f\u7528\u4e8e\u63a2\u7d22\u5b54\u9053\u4e2d\u7684\u53cd\u5e94\u4f4d\u70b9\u3002\u901a\u8fc7\u63a7\u52361D\u901a\u9053\u957f\u5ea6\uff08\u22640.59 \u03bcm\uff09\uff0c\u4f5c\u8005\u53d1\u73b0\u5fae\u5b54\u9053\u9650\u5236\u6fc0\u5b50\u5728\u5149\u50ac\u5316\u4e2d\u8d77\u4e3b\u5bfc\u4f5c\u7528\uff0c\u5e76\u663e\u8457\u63d0\u9ad8\u4e86H<sub>2<\/sub>\u7684\u6790\u51fa\u901f\u7387\uff0c\u6700\u9ad8\u8fbe\u5230358 mmol h<sup>\u22121<\/sup>\u00a0g<sup>\u22121<\/sup>\uff08537 \u03bcmol h<sup>\u22121<\/sup>\uff09\uff0c420 nm\u5904\u7684\u8868\u89c2\u91cf\u5b50\u4ea7\u7387\uff08AQY\uff09\u4e3a28.6%\u3002\u5728\u53ef\u6269\u5c55\u7684\u5e73\u677f\u53cd\u5e94\u5668\u4e2d\uff0c\u5728\u8f90\u7167\uff081000 W m<sup>\u22122<\/sup>\uff099 h\u5185\uff0c\u6bcf\u5e73\u65b9\u7c73\u8d1f\u8f7dHOF-H<sub>4<\/sub>TBAPy\u7684\u7ea4\u7ef4\u6536\u96c6\u4e86\u8d85\u8fc71 mol H<sub>2<\/sub>\u3002\u56e0\u6b64\uff0c\u901a\u8fc7\u6784\u5efa\u53ef\u63a5\u8fd1\u76841D\u5fae\u5b54\u9053\u6765\u9650\u5236\u6fc0\u5b50\uff0c\u4e3a\u589e\u5f3a\u6709\u673a\u534a\u5bfc\u4f53\u7684\u5149\u6d3b\u6027\u63d0\u4f9b\u4e86\u4e00\u79cd\u65b0\u9014\u5f84\u3002<\/section>\n<p>&nbsp;<\/p>\n<p><img decoding=\"async\" title=\"1\" src=\"http:\/\/9794.seohost.cn\/storage\/9794\/article\/20230620\/1687229579756489.jpg\" alt=\"1\" \/><\/p>\n<p>&nbsp;<\/p>\n<section data-role=\"title\" data-tools=\"135\u7f16\u8f91\u5668\" data-id=\"us-4152855\">\n<section>\n<section>\n<section>\n<section data-brushtype=\"text\"><strong>\u7814\u7a76\u80cc\u666f<\/strong><\/section>\n<\/section>\n<\/section>\n<\/section>\n<\/section>\n<section>\u6709\u673a\u534a\u5bfc\u4f53\u5149\u50ac\u5316\u5242\u56e0\u5176\u7535\u5b50\u6027\u8d28\u6613\u4e8e\u901a\u8fc7\u5206\u5b50\u5de5\u7a0b\u8fdb\u884c\u8c03\u8282\uff0c\u53d7\u5230\u4e86\u5e7f\u6cdb\u5173\u6ce8\u3002\u7136\u800c\uff0c\u5927\u591a\u6570\u6709\u673a\u534a\u5bfc\u4f53\u7684\u6fc0\u5b50\u6269\u6563\u957f\u5ea6\u8f83\u77ed\uff08\u901a\u5e38\u4e3a5-10 nm\uff09\u5bfc\u81f4\u4e86\u8f83\u9ad8\u7684\u91cd\u7ec4\u7387\u548c\u8f83\u5dee\u7684\u6fc0\u5b50\u89e3\u79bb\u3002\u76ee\u524d\u62a5\u9053\u7684\u6709\u673a\u534a\u5bfc\u4f53\u4e2d\u4ea7\u751f\u7684\u5927\u591a\u6570\u7535\u8377\u65e0\u6cd5\u8fc1\u79fb\u5230\u8868\u9762\u8fdb\u884c\u6c27\u5316\u8fd8\u539f\u53cd\u5e94\uff0c\u7279\u522b\u662f\u5728\u8f83\u5927\u7c92\u5f84\u4e0b\u3002\u6700\u8fd1\uff0c\u79d1\u7814\u4eba\u5458\u96c6\u4e2d\u5728\u4f7f\u7528\u7eb3\u7c73\u9897\u7c92\u3001\u4f9b\u4f53\/\u53d7\u4f53\u5f02\u8d28\u7ed3\u548c\u6709\u673a\u591a\u5b54\u805a\u5408\u7269\u6765\u6539\u5584\u5149\u50ac\u5316\u5242\u7684\u6fc0\u5b50\u89e3\u79bb\uff0c\u56e0\u6b64\u786e\u5b9a\u6fc0\u5b50\u79bb\u89e3\u754c\u9762\u5e76\u63a2\u7d22\u5176\u79bb\u89e3\u673a\u5236\u662f\u5f00\u53d1\u9ad8\u6027\u80fd\u6709\u673a\u5149\u50ac\u5316\u5242\u7684\u57fa\u7840\u3002<\/section>\n<section>\u8fd1\u5e74\u6765\uff0c\u6c22\u952e\u6709\u673a\u9aa8\u67b6HOF-H<sub>4<\/sub>TBAPy\u5177\u6709\u72ec\u7279\u7684\u6027\u8d28\uff0c\u5f15\u8d77\u4e86\u5149\u5316\u5b66\u9886\u57df\u7684\u5e7f\u6cdb\u5173\u6ce8\u3002\u7814\u7a76\u8868\u660e\uff0c\u5206\u5b50\u6676\u4f53\u4e2d\u7684\u6676\u4f53\u5806\u79ef\u4f1a\u5f71\u54cd\u5149\u50ac\u5316\u6d3b\u6027\u3002\u4f46\u662f\uff0c\u8fd9\u79cd\u72ec\u7279\u7684\u5b54\u7ed3\u6784\u5bf9\u5149\u50ac\u5316\u4e2d\u6fc0\u5b50\u8fc1\u79fb\u548c\u5b54\u9650\u5236\u53cd\u5e94\u7684\u5f71\u54cd\u8fd8\u4e0d\u6e05\u695a\u3002\u6b64\u5916\uff0c\u9610\u660e\u591a\u5b54\u6709\u673a\u534a\u5bfc\u4f53\u7684\u7ed3\u6784-\u7535\u5b50\u6027\u8d28\u5173\u7cfb\u8fd8\u5177\u6709\u6311\u6218\u6027\u3002\u5982\u679c\u5b54\u9053\u53ef\u63a5\u8fd1\uff0c\u5149\u751f\u6fc0\u5b50\u901a\u5e38\u53ea\u9700\u8981\u8fc1\u79fb\u51e0\u7eb3\u7c73\u5c31\u80fd\u5230\u8fbe\u5b54\u9053\u5185\u8868\u9762\uff0c\u4ece\u800c\u89e3\u79bb\u5e76\u9a71\u52a8\u6c27\u5316\u8fd8\u539f\u53cd\u5e94\u3002\u8d85\u77ed\u7684\u8f6c\u79fb\u8def\u5f84\u51cf\u5c11\u4e86\u7535\u8377\u635f\u5931\uff0c\u6709\u5229\u4e8e\u50ac\u5316\u53cd\u5e94\u3002<\/section>\n<section data-role=\"title\" data-tools=\"135\u7f16\u8f91\u5668\" data-id=\"us-4152855\">\n<section>\n<section>\n<section>\n<section data-brushtype=\"text\"><strong>\u56fe\u6587\u5bfc\u8bfb<\/strong><\/section>\n<\/section>\n<\/section>\n<\/section>\n<\/section>\n<section>\u4f5c\u8005\u901a\u8fc7\u8c03\u6574H<sub>4<\/sub>TBAPy\u5728\u6eb6\u5242\u76f8\u4e2d\u7684\u6c89\u6dc0\u6761\u4ef6\uff0c\u5f97\u5230\u4e86HOF-H<sub>4<\/sub>TBAPy\u3002\u5bf9\u6bd4\u6eb6\u5242\u6cd5\uff0c\u8be5\u65b9\u6cd5\u5728\u6676\u4f53\u751f\u957f\u8fc7\u7a0b\u4e2d\u5177\u6709\u53ef\u63a7\u7684\u8131\u8d28\u5b50\u4f5c\u7528\u3002<\/section>\n<section>\u975e\u5c40\u90e8\u5bc6\u5ea6\u6cdb\u51fd\u7406\u8bba\uff08NLDFT\uff09\u6a21\u578b\u62df\u5408N<sub>2<\/sub>\u7b49\u6e29\u7ebf\u7684\u5e73\u5747\u5b54\u9699\u5206\u5e03\u4e3a1.5 nm\u3002\u6b64\u5916\uff0c\u7c89\u672bX\u5c04\u7ebf\u884d\u5c04\uff08PXRD\uff09\u56fe\u4e2d(011)\u6676\u97624.26\u00b0\u9644\u8fd1\u7684\u8868\u89c2\u884d\u5c04\u5cf0\uff0c\u8bc1\u660e\u4e86HOF-H<sub>4<\/sub>TBAPy\u7ed3\u6784\u4e2d\u5b58\u5728\u9ad8\u5ea6\u6709\u5e8f\u7684\u5fae\u5b54\u3002\u5728\u7eb3\u7c73\u68d2\u72b6HOF-H<sub>4<\/sub>TBAPy\u4e0a\u89c2\u5bdf\u52302.06 nm\u7684\u9ad8\u6709\u5e8f\u6761\u7eb9\u5206\u5e03\uff0c\u5bf9\u5e94\u4e8e\u6709\u5e8f\u76841D\u901a\u9053\u72b6\u5b54\u9699\u3002\u7ed3\u679c\u8868\u660e\uff0cHOF-H<sub>4<\/sub>TBAPy\u662f\u4e00\u4e2a\u7531H<sub>4<\/sub>TBAP\u6784\u5efa\u7684\u5177\u6709\u6709\u5e8f\u5fae\u5b54\u7ed3\u6784\u7684\u6c22\u952e\u6709\u673a\u9aa8\u67b6\u3002<\/section>\n<section><img decoding=\"async\" title=\"2\" src=\"http:\/\/9794.seohost.cn\/storage\/9794\/article\/20230620\/1687229589639349.jpg\" alt=\"2\" \/><\/section>\n<section><strong>\u56fe1.HOF-H<sub>4<\/sub>TBAPy\u7684\u7ed3\u6784<\/strong><\/section>\n<section><img decoding=\"async\" title=\"3\" src=\"http:\/\/9794.seohost.cn\/storage\/9794\/article\/20230620\/1687229596798046.jpg\" alt=\"3\" \/><\/section>\n<section><strong>\u56fe2.\u8d85\u5feb\u5149\u8c31\u63a2\u6d4b\u9650\u5236\u5728\u5fae\u5b54\u5185\u7684\u6fc0\u5b50\u8f6c\u79fb<\/strong><\/section>\n<section>\u5728298.15 K\u4e0b\uff0cHOF-H<sub>4<\/sub>TBAPy\u53ef\u5b9e\u73b0\u9ad8\u8fbe44.7 wt%\u7684\u53ef\u9006\u5438\u9644\uff0c\u800cH<sub>4<\/sub>TBAPy\u4ec5\u5438\u9644\u4e8611.47 wt%\u7684\u6c34\uff0c\u5e76\u4e14\u8868\u73b0\u51fa\u6709\u9650\u7684\u4eb2\u6c34\u6027\u3002\u968f\u7740HOF-H<sub>4<\/sub>TBAPy\u7684\u5e73\u5747\u957f\u5ea6\u9010\u6e10\u51cf\u5c0f\uff0c\u5176\u4e0e\u6c34\u7684\u63a5\u89e6\u89d2\u4ece34.50\u00b0\u51cf\u5c0f\u523011.85\u00b0\u3002\u968f\u77401D\u5b54\u9053\u957f\u5ea6\u7684\u9010\u6e10\u589e\u52a0\uff0c\u5149\u6d3b\u6027\u5148\u4fdd\u6301\u4e0d\u53d8\uff0c\u7136\u540e\u4ee5\u8fd1\u4f3c\u53cd\u6bd4\u7684\u65b9\u5f0f\u4e0b\u964d\uff0c\u8bc1\u5b9e\u4e86\u5fae\u5b54\u9650\u57df\u6fc0\u5b50\u9a71\u52a8\u4e86\u5149\u6d3b\u6027\uff0c\u5e76\u4e14\u5f3a\u70c8\u4f9d\u8d56\u4e8e\u5fae\u5b54\u5185\u90e8\u7684\u826f\u597d\u63a5\u89e6\u3002<\/section>\n<section><img decoding=\"async\" title=\"4\" src=\"http:\/\/9794.seohost.cn\/storage\/9794\/article\/20230620\/1687229604481655.jpg\" alt=\"4\" 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mmol h<sup>\u22121<\/sup>\u00a0g<sup>\u22121<\/sup>\u3002<\/section>\n<section><img decoding=\"async\" title=\"5\" src=\"http:\/\/9794.seohost.cn\/storage\/9794\/article\/20230620\/1687229613722703.jpg\" alt=\"5\" \/><\/section>\n<section><strong>\u56fe4. \u5fae\u5b54\u4e2d\u53cd\u5e94\u4f4d\u70b9\u7684\u9274\u5b9a<\/strong><\/section>\n<section><img decoding=\"async\" title=\"7\" src=\"http:\/\/9794.seohost.cn\/storage\/9794\/article\/20230620\/1687229624103285.jpg\" alt=\"7\" \/><\/section>\n<section><strong>\u56fe5. HOF-H<sub>4<\/sub>TBAPy\u7684\u5149\u50ac\u5316\u6790\u6c22\u6027\u80fd<\/strong><\/section>\n<section data-role=\"title\" data-tools=\"135\u7f16\u8f91\u5668\" data-id=\"us-4152855\">\n<section>\n<section>\n<section>\n<section data-brushtype=\"text\"><strong>\u6587\u732e\u4fe1\u606f<\/strong><\/section>\n<\/section>\n<\/section>\n<\/section>\n<\/section>\n<section>Photocatalytic sacrificial H<sub>2<\/sub>\u00a0evolution dominated by micropore-confined exciton transfer in hydrogen-bonded organic frameworks.\u00a0<em>Nature Catalysis<\/em>,\u00a0<strong>2023<\/strong>, DOI: https:\/\/doi.org\/10.1038\/s41929-023-00972-x.<\/section>\n<p>&nbsp;<\/p>\n","protected":false},"excerpt":{"rendered":"<p>\u6210\u679c\u7b80\u4ecb &nbsp; \u6709\u673a\u534a\u5bfc\u4f53\uff08organic semiconductors\uff09\u662f\u4e00\u7c7b\u5341\u5206\u5177\u6709\u5438\u5f15\u529b\u7684\u5149\u50ac\u5316 [&hellip;]<\/p>\n","protected":false},"author":326,"featured_media":0,"comment_status":"open","ping_status":"open","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[14],"tags":[],"class_list":["post-48415","post","type-post","status-publish","format-standard","hentry","category-tuijianyuedu"],"_links":{"self":[{"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/posts\/48415","targetHints":{"allow":["GET"]}}],"collection":[{"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/posts"}],"about":[{"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/users\/326"}],"replies":[{"embeddable":true,"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/comments?post=48415"}],"version-history":[{"count":1,"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/posts\/48415\/revisions"}],"predecessor-version":[{"id":48416,"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/posts\/48415\/revisions\/48416"}],"wp:attachment":[{"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/media?parent=48415"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/categories?post=48415"},{"taxonomy":"post_tag","embeddable":true,"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/tags?post=48415"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}