{"id":48248,"date":"2023-06-17T08:09:52","date_gmt":"2023-06-17T00:09:52","guid":{"rendered":"https:\/\/www.chemhui.com\/?p=48248"},"modified":"2023-05-31T10:10:21","modified_gmt":"2023-05-31T02:10:21","slug":"%e9%99%88%e5%ae%9c%e6%b3%95-%e8%be%9b%e5%bf%97%e5%b3%b0adv-sci-%ef%bc%9afe%e8%bf%91100%ef%bc%81hmtamof-545-co%e5%8a%a9%e5%8a%9b%e5%85%89%e8%be%85%e5%8a%a9co2%e7%94%b5%e8%bf%98%e5%8e%9f","status":"publish","type":"post","link":"http:\/\/www.chemhui.com\/%e9%99%88%e5%ae%9c%e6%b3%95-%e8%be%9b%e5%bf%97%e5%b3%b0adv-sci-%ef%bc%9afe%e8%bf%91100%ef%bc%81hmtamof-545-co%e5%8a%a9%e5%8a%9b%e5%85%89%e8%be%85%e5%8a%a9co2%e7%94%b5%e8%bf%98%e5%8e%9f\/","title":{"rendered":"\u9648\u5b9c\u6cd5\/\u8f9b\u5fd7\u5cf0Adv. Sci.\uff1aFE\u8fd1100%\uff01HMTA@MOF-545-Co\u52a9\u529b\u5149\u8f85\u52a9CO2\u7535\u8fd8\u539f"},"content":{"rendered":"
\u9ad8\u6548\u7684CO2<\/sub>\u7535\u8fd8\u539f\u6210\u9ad8\u4ef7\u503c\u4ea7\u54c1\u5728\u5f88\u5927\u7a0b\u5ea6\u4e0a\u4f9d\u8d56\u4e8eCO2<\/sub>\u7684\u5438\u9644\/\u6d3b\u5316\u6216\u7535\u50ac\u5316\u5242\u7684\u7535\u5b50\u8f6c\u79fb\uff0c\u975e\u5e38\u9700\u8981\u80fd\u591f\u4fc3\u8fdb\u7535\u50ac\u5316\u5242\u76f8\u4e92\u4f5c\u7528\u7684\u7279\u5b9a\u4f4d\u70b9\u529f\u80fd\u5316\u65b9\u6cd5\u3002<\/section>\n

 <\/p>\n

\u57fa\u4e8e\u6b64\uff0c\u534e\u5357\u5e08\u8303\u5927\u5b66\u9648\u5b9c\u6cd5\u6559\u6388\u548c\u5b89\u5fbd\u5de5\u4e1a\u5927\u5b66\u8f9b\u5fd7\u5cf0\u526f\u6559\u6388\u7b49\u4eba<\/strong>\u62a5\u9053\u4e86\u4e00\u79cd\u5b9a\u5411\u914d\u4f4d\u7b56\u7565\uff0c\u5c06\u5bccN\u52a9\u5242\uff08\u516d\u4e9a\u7532\u57fa\u56db\u80fa\uff0cHMTA\uff09\u5f15\u5165\u5230\u91d1\u5c5e\u535f\u5549\u91d1\u5c5e\u6709\u673a\u6846\u67b6\uff08MOFs\uff09\u4e2d\uff0c\u5408\u6210\u4e86\u4e00\u7cfb\u5217\u4f4d\u70b9\u7279\u5f02\u6027\u529f\u80fd\u5316\u7535\u50ac\u5316\u5242\uff08HMTA@MOF-545-M\uff0cM=Fe\u3001Co\u3001Ni\uff09\uff0c\u5e76\u6210\u529f\u5e94\u7528\u4e8e\u5149\u8f85\u52a9CO2<\/sub>\u7535\u8fd8\u539f\u4e2d\u3002<\/section>\n
\u5176\u4e2d\uff0cHMTA@MOF-545-Co\u5728\u5149\u7167\u6761\u4ef6\u4e0b\uff0c\u5176CO2<\/sub>\u7535\u8fd8\u539f\u7684\u6cd5\u62c9\u7b2c\u6548\u7387\uff08FECO<\/sub>\uff09\u7ea6100%\u3001CO\u751f\u6210\u901f\u7387\u7ea65.11 mol m\u22122<\/sup>\u00a0h\u22121<\/sup>\u548c\u80fd\u91cf\u6548\u7387\u7ea670%\u3002<\/section>\n
\"1\"<\/section>\n
\u901a\u8fc7DFT\u8ba1\u7b97\uff0c\u4f5c\u8005\u7814\u7a76\u4e86HMTA@MOF-545-Co\u7684\u7535\u50ac\u5316CO2<\/sub>RR\u673a\u7406\u3002HMTA\u4e0eHMTA@MOF-545-Co\u4e2d\u7684Co-TCPP\u5355\u5143\u5177\u6709\u8f83\u5f3a\u7684\u76f8\u4e92\u4f5c\u7528\uff0c\u53ef\u4ee5\u663e\u8457\u63d0\u9ad8\u6d3b\u6027\u4f4d\u70b9\u7684\u7535\u8377\u5bc6\u5ea6\u3002HMTA\u4e0eCo-TCPP\u4e4b\u95f4\u7684\u952e\u957f\u5728\u914d\u4f4d\u952e\u8303\u56f4\u5185\uff0c\u8868\u660eHMTA\u4e0eCo-TCPP\u7684Co\u539f\u5b50\u901a\u8fc7\u914d\u4f4d\u952e\u8fde\u63a5\u3002\u540c\u65f6\uff0c\u4f5c\u8005\u8fd8\u8ba1\u7b97\u4e86CO2<\/sub>RR\u8fc7\u7a0b\u5404\u6b65\u9aa4\u50ac\u5316\u5242\u4e0a\u4e2d\u95f4\u4f53\u7684\u7406\u8bba\u6a21\u578b\u3002<\/section>\n
\u4e00\u822c\u800c\u8a00\uff0cCO2<\/sub>\u8f6c\u5316\u4e3aCO\u7684\u8f6c\u5316\u8fc7\u7a0b\u5305\u62ec\uff1aCO2<\/sub>\u5438\u9644\/\u6d3b\u5316\u751f\u6210*CO2<\/sub>\uff0c\u8f6c\u5316\u4e3a*COOH\uff0c\u518d\u8f6c\u5316\u4e3a*CO\uff0c\u6700\u540e\u662fCO\u89e3\u5438\u5728MOF-545-Co\u7684\u60c5\u51b5\u4e0b\uff0cCO2<\/sub>\u5206\u5b50\u4e0eCo-TCPP\u7684\u76f8\u4e92\u4f5c\u7528\u529b\u8f83\u5f31\uff0c\u7ed3\u5408\u80fd\u4ec5\u4e3a-0.31 eV\u3002<\/section>\n
\"2\"<\/section>\n
\u6b64\u5916\uff0c\u8ba1\u7b97\u51fa\u5438\u9644\u7684*CO2<\/sub>\u5230*COOH\u7684\u5409\u5e03\u65af\u81ea\u7531\u80fd\u4e3a1.04 eV\uff0c\u4e5f\u662fCO\u751f\u6210\u7684\u51b3\u5b9a\u6b65\u9aa4\uff0c\u7136\u540e*COOH\u8f6c\u5316\u4e3a*CO\uff0c\u6700\u7ec8\u5728MOF-545-Co\u4e0a\u8fdb\u884cCO\u89e3\u5438\u9700\u89810.49 eV\u3002\u5bf9\u4e8eHMTA@MOF-545-Co\uff0cHMTA\u6539\u6027\u540e\uff0cCO2<\/sub>\u5438\u9644\u80fd\u5927\u5e45\u63d0\u9ad8\uff0c\u8fbe\u5230-0.53 eV\uff0c\u51e0\u4e4e\u7ffb\u500d\u589e\u5f3a\u3002\u7136\u540e*COOH\u8f6c\u5316\u4e3a*CO\u53ea\u9700\u8981-0.14 eV\u7684\u80fd\u91cf\uff0c\u6700\u540e*CO\u7ecf\u8fc7\u89e3\u5438\u8fc7\u7a0b\u751f\u6210CO\u3002<\/section>\n
\u56e0\u6b64\uff0cHMTA\u7684\u5f15\u5165\u4e0eMOF-545-Co\u4ea7\u751f\u5f3a\u914d\u952e\uff0c\u53ef\u589e\u52a0\u6d3b\u6027\u4f4d\u70b9\u7684\u7535\u8377\u5bc6\u5ea6\uff0c\u51e0\u4e4e\u52a0\u500d\u63d0\u9ad8CO2<\/sub>\u5438\u9644\u80fd\uff0c\u5e76\u6781\u5927\u964d\u4f4e\u901f\u7387\u51b3\u5b9a\u6b65\u9aa4\u7684\u80fd\u5792\uff0c\u4ece\u800c\u63d0\u9ad8CO2<\/sub>RR\u6027\u80fd\u3002<\/section>\n
\"3\"<\/section>\n
Electronic Tuning of CO2<\/sub>\u00a0Interaction by Oriented Coordination of N-Rich Auxiliary in Porphyrin Metal-Organic Frameworks for Light-Assisted CO2<\/sub>\u00a0Electroreduction.\u00a0Adv. Sci.,\u00a0<\/em>2023<\/strong>, DOI: 10.1002\/advs.202301261.<\/section>\n
https:\/\/doi.org\/10.1002\/advs.202301261.<\/section>\n
\n
\n
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<\/section>\n<\/section>\n<\/section>\n<\/section>\n

 <\/p>\n","protected":false},"excerpt":{"rendered":"

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