{"id":48194,"date":"2023-06-09T08:15:56","date_gmt":"2023-06-09T00:15:56","guid":{"rendered":"https:\/\/www.chemhui.com\/?p=48194"},"modified":"2023-05-25T10:16:45","modified_gmt":"2023-05-25T02:16:45","slug":"%e6%b1%9f%e8%a5%bf%e5%b8%88%e8%8c%83%e5%a4%a7%e5%ad%a6%e8%a2%81%e5%bd%a9%e9%9b%b7%e6%95%99%e6%8e%88%e5%9b%a2%e9%98%9fadvanced-materials%ef%bc%9a%e4%ba%8c%e7%bb%b4mos2%e5%b1%82%e9%97%b4%e9%99%90","status":"publish","type":"post","link":"http:\/\/www.chemhui.com\/%e6%b1%9f%e8%a5%bf%e5%b8%88%e8%8c%83%e5%a4%a7%e5%ad%a6%e8%a2%81%e5%bd%a9%e9%9b%b7%e6%95%99%e6%8e%88%e5%9b%a2%e9%98%9fadvanced-materials%ef%bc%9a%e4%ba%8c%e7%bb%b4mos2%e5%b1%82%e9%97%b4%e9%99%90\/","title":{"rendered":"\u6c5f\u897f\u5e08\u8303\u5927\u5b66\u8881\u5f69\u96f7\u6559\u6388\u56e2\u961fAdvanced Materials\uff1a\u4e8c\u7ef4MoS2\u5c42\u95f4\u9650\u57dfNiFe\u53cc\u539f\u5b50\u63d0\u5347\u9178\u6027\u5168\u89e3\u6c34\u6027\u80fd"},"content":{"rendered":"<section>\u7a7a\u95f4\u9650\u57df\u7b56\u7565\u662f\u5c06\u6d3b\u6027\u7269\u79cd\u9650\u5236\u6216\u5c01\u88c5\u5728\u7eb3\u7c73\u6216\u4e9a\u7eb3\u7c73\u7a7a\u95f4\u4e2d\u4ee5\u63d0\u4f9b\u5e73\u8861\u8fc7\u6e21\u6001\u7684\u72ec\u7279\u5fae\u73af\u5883\u6765\u8c03\u8282\u5316\u5b66\u53cd\u5e94\u7684\u7b56\u7565\u3002\u9650\u57df\u5fae\u73af\u5883\u4e0d\u4ec5\u53ef\u4ee5\u6291\u5236\u6d3b\u6027\u4f4d\u70b9\u53ef\u80fd\u51fa\u73b0\u7684\u56e2\u805a\u548c\u6c27\u5316\u95ee\u9898\uff0c\u8fd8\u4f7f\u5f97\u4e2d\u95f4\u4ea7\u7269\u3001\u53cd\u5e94\u7269\u548c\u4ea7\u7269\u5728\u9650\u57df\u7a7a\u95f4\u5185\u66f4\u5bb9\u6613\u8f6c\u79fb\uff0c\u53ef\u4ee5\u5b9e\u73b0\u50ac\u5316\u5242\u7684\u9ad8\u6d3b\u6027\u3001\u9ad8\u9009\u62e9\u6027\u548c\u9ad8\u7a33\u5b9a\u6027\uff0c\u4e3a\u5f02\u8d28\u50ac\u5316\u63d0\u4f9b\u4e86\u4e00\u4e2a\u6709\u5438\u5f15\u529b\u7684\u50ac\u5316\u5e73\u53f0\u3002\u503c\u5f97\u4e00\u63d0\u7684\u662f\uff0c\u5c42\u72b6\u4e8c\u7ef4\u6750\u6599\u5728\u6784\u5efa\u9650\u57df\u7ed3\u6784\u9886\u57df\u8868\u73b0\u51fa\u5de8\u5927\u7684\u6f5c\u529b\uff0c\u5176\u5185\u5728\u7684\u5177\u6709\u8303\u5fb7\u74e6\u5c14\u65af\u76f8\u4e92\u4f5c\u7528\u7684\u5c42\u95f4\u533a\u57df\uff0c\u4e0d\u4ec5\u662f\u4e00\u79cd\u6709\u524d\u9014\u7684\u9650\u57df\u7a7a\u95f4\uff0c\u540c\u65f6\u4e5f\u53ef\u80fd\u4f1a\u662f\u7a33\u5b9a\u529f\u80fd\u6027\u5ba2\u4f53\u6750\u6599\uff08\u5982\u91d1\u5c5e\u3001\u805a\u5408\u7269\u3001\u6709\u673a\u5c0f\u5206\u5b50\u7b49\uff09\u7684\u7eb3\u7c73\u201c\u5e87\u62a4\u6240\u201d\u3002<\/section>\n<p>&nbsp;<\/p>\n<section>\u53e6\u4e00\u65b9\u9762\uff0c\u53cc\u5355\u539f\u5b50\u50ac\u5316\u5242\u4f5c\u4e3a\u5355\u539f\u5b50\u50ac\u5316\u5242\u7684\u5ef6\u4f38\uff0c\u5728\u534f\u540c\u9a71\u52a8\u66f4\u590d\u6742\u7684\u591a\u6b65\u50ac\u5316\u53cd\u5e94\u65b9\u9762\u5177\u6709\u660e\u663e\u4f18\u52bf\uff0c\u5df2\u7ecf\u6210\u4e3a\u7535\u50ac\u5316\u3001\u5149\u50ac\u5316\u53ca\u80fd\u6e90\u5b58\u50a8\u7b49\u9886\u57df\u7684\u7814\u7a76\u70ed\u70b9\u3002\u56e0\u6b64\uff0c\u5728\u4e8c\u7ef4\u5c42\u72b6\u6750\u6599\u7684\u8303\u5fb7\u534e\u95f4\u9699\u4e2d\u63d2\u5165\u53cc\u539f\u5b50\u7269\u79cd\u4f5c\u4e3a\u5ba2\u4f53\u6750\u6599\uff0c\u5c06\u6709\u671b\u5728\u4fdd\u6301\u53cc\u539f\u5b50\u7269\u79cd\u4f18\u5f02\u7279\u6027\u7684\u57fa\u7840\u4e0a\u8fdb\u4e00\u6b65\u4f18\u5316\u4e2d\u95f4\u4f53\u7684\u5438\u9644\u5f3a\u5ea6\uff0c\u5927\u5927\u52a0\u5feb\u50ac\u5316\u52a8\u529b\u5b66\u3002\u540c\u65f6\uff0c\u7a7a\u95f4\u9650\u57df\u7684\u7ed3\u6784\u4e5f\u53ef\u4ee5\u5f88\u597d\u5730\u4fdd\u62a4\u5177\u6709\u6781\u9ad8\u8868\u9762\u81ea\u7531\u80fd\u7684\u53cc\u5355\u539f\u5b50\u514d\u4e8e\u70ed\u529b\u5b66\u9a71\u4f7f\u7684\u539f\u5b50\u56e2\u805a\u3001\u8150\u8680\u7b49\u635f\u5bb3\u50ac\u5316\u5242\u6027\u80fd\u7684\u95ee\u9898\u3002\u7136\u800c\uff0c\u4ece\u8bbe\u8ba1\u548c\u5408\u6210\u7684\u89d2\u5ea6\u6765\u770b\uff0c\u5728\u4e8c\u7ef4\u5c3a\u5ea6\u4e0a\uff0c\u5c06\u53cc\u5355\u539f\u5b50\u7cbe\u786e\u7ec4\u88c5\u5728\u4e24\u4e2a\u76f8\u90bb\u7684\u5c42\u95f4\u662f\u6781\u5177\u6311\u6218\u6027\u7684\u3002<\/section>\n<section>\u8fd1\u671f\uff0c<strong>\u6c5f\u897f\u5e08\u8303\u5927\u5b66\u8881\u5f69\u96f7\u6559\u6388\u56e2\u961f<\/strong>\u9996\u6b21\u63d0\u51fa\u4e86\u4e00\u4e2a\u65b0\u7684\u5c42\u95f4\u9650\u57df\u7b56\u7565\uff0c<\/section>\n<section>\u5728\u4e8c\u7ef4\u5c3a\u5ea6\u4e0a\u540c\u65f6\u5c06\u4e24\u79cd\u5355\u539f\u5b50\u951a\u5b9a\u5728MoS<sub>2<\/sub>\u7684\u5c42\u95f4\uff0c\u4f7f\u5176\u4e0d\u4f46\u7ee7\u627f\u4e86\u53cc\u5355\u539f\u5b50\u7269\u79cd\u7684\u9ad8\u6d3b\u6027\u4f18\u52bf\uff0c\u8fd8\u4f7f\u5f97\u8be5\u9650\u57df\u578b\u50ac\u5316\u5242\u8868\u73b0\u51fa\u66f4\u4f18\u5f02\u7684\u5438\u9644\u5e73\u8861\u3001\u672c\u5f81\u6d3b\u6027\u53ca\u5bfc\u7535\u6027\uff1b\u540c\u65f6\uff0c\u5c42\u95f4\u9650\u57df\u7ed3\u6784\u4e5f\u663e\u8457\u63d0\u5347\u4e86\u50ac\u5316\u5242\uff08\u5305\u62ec\u91d1\u5c5e\u53cc\u5355\u539f\u5b50\uff09\u7684\u7a33\u5b9a\u6027\uff08\u6ce8\uff1a\u5373\u4f7f\u5728\u6076\u52a3\u7684\u9178\u6027\u73af\u5883\u4e2d\uff0c\u8be5\u9650\u57df\u578b\u50ac\u5316\u5242\u7684\u6027\u80fd\u4e5f\u80fd\u591f\u7a33\u5065\u63d0\u5347\uff09\uff0c\u4ece\u800c\u83b7\u5f97\u4e86\u5728\u9178\u6027\u6761\u4ef6\u4e0b\u9ad8\u6548\u4e14\u7a33\u5b9a\u7684\u4f4e\u6210\u672c\u5168\u89e3\u6c34\u7535\u50ac\u5316\u5242\u3002\u7406\u8bba\u8ba1\u7b97\u548c\u5b9e\u9a8c\u7ed3\u679c\u8868\u660e\uff0c\u9650\u57df\u7ed3\u6784\u5bf9\u4e8e\u8fd9\u79cd\u53cc\u529f\u80fdNiFe\u53cc\u5355\u539f\u5b50\u50ac\u5316\u5242\u5728\u9ad8\u6548\u4fc3\u8fdb\u6c34\u5206\u89e3\u8fc7\u7a0b\u548c\u4fdd\u62a4\u53cc\u5355\u539f\u5b50\u8fdc\u79bb\u82db\u523b\u7684\u9178\u6027\u6761\u4ef6\u65b9\u9762\u8d77\u5230\u4e86\u5173\u952e\u6027\u4f5c\u7528\u3002\u8be5\u7814\u7a76\u7cfb\u7edf\u5730\u9610\u91ca\u4e86\u539f\u5b50\u6c34\u5e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NiFe Dual Atoms within MoS<sub>2<\/sub>\u00a0Electrocatalyst for Ultra-Efficient Acidic Overall Water Splitting\u300b\u4e3a\u9898\u5728\u7ebf\u53d1\u8868\u5728\u300aAdvanced Materials\u300b\u3002\u6c5f\u897f\u5e08\u8303\u5927\u5b66\u4e3a\u7b2c\u4e00\u5b8c\u6210\u5355\u4f4d\u5e76\u4e14\u662f\u552f\u4e00\u901a\u8baf\u5355\u4f4d\uff0c\u8881\u5f69\u96f7\u6559\u6388\u4e3a\u672c\u6587\u552f\u4e00\u901a\u8baf\u4f5c\u8005\u3002\u8be5\u9879\u5de5\u4f5c\u5f97\u5230\u4e86\u56fd\u5bb6\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u59d4\u3001\u6c5f\u897f\u7701\u4e3b\u8981\u5b66\u79d1\u5b66\u672f\u548c\u6280\u672f\u5e26\u5934\u4eba\u57f9\u517b\u8ba1\u5212\u2014\u9886\u519b\u4eba\u624d\u9879\u76ee\u4ee5\u53ca\u6c5f\u897f\u7701\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u59d4\u7b49\u7684\u652f\u6301\u3002<\/section>\n<section><img decoding=\"async\" title=\"1\" src=\"http:\/\/9794.seohost.cn\/storage\/9794\/article\/20230514\/1684027513597050.jpg\" alt=\"1\" \/><\/section>\n<section><strong>\u56fe1<\/strong>. \uff08a\uff09\u5728\u4e8c\u7ef4\u5c3a\u5ea6\u4e0a\u539f\u5b50\u7ea7\u5730\u7ec4\u88c5\u5c42\u95f4\u9650\u57df\u53cc\u5355\u539f\u5b50\u50ac\u5316\u5242\u7684\u8bbe\u60f3\uff1bDFT\u6a21\u578b\uff08b\uff09\u5e73\u9762NiFe@MoS<sub>2<\/sub>\uff0c\uff08c\uff091.5 nm\u5c42\u95f4\u9650\u57df\u7684NiFe@MoS<sub>2<\/sub>\u548c\uff08d\uff091.2 nm\u5c42\u95f4\u9650\u57df\u7684NiFe@MoS<sub>2<\/sub>\uff1b\uff08e\uff09\u6c34\u89e3\u79bb\u8fc7\u7a0b\u7684\u80fd\u91cf\u6bd4\u8f83\uff1b\uff08f\uff09\u6790\u6c22\u53cd\u5e94\u8fc7\u7a0b\u7684\u81ea\u7531\u80fd\u56fe\u3002<\/section>\n<section><img decoding=\"async\" title=\"2\" src=\"http:\/\/9794.seohost.cn\/storage\/9794\/article\/20230514\/1684027522999643.jpg\" alt=\"2\" \/><\/section>\n<section><strong>\u56fe2<\/strong>. \u57281.2nm\u5c42\u95f4\u9650\u57df\u7684NiFe@MoS<sub>2<\/sub>\u7684\uff08a\uff09Ni\u4f4d\u70b9\u548c\uff08b\uff09Fe\u4f4d\u70b9\u7684\u9178\u6027\u6790\u6c27\u53cd\u5e94\u673a\u7406\u56fe\uff1b\uff08c\uff09\u6790\u6c27\u53cd\u5e94\u5728\u5b9a\u7535\u4f4d\u4e3a1.23 V\u65f6\u7684\u8def\u5f84\u56fe\uff0c\u5176\u4e2d\u51b3\u901f\u6b65\u9aa4\u7528\u5404\u81ea\u989c\u8272\u5bf9\u5e94\u7684\u661f\u5f62\u6807\u8bb0;\uff08d\uff091.5 nm\u5c42\u95f4\u9650\u57dfNiFe@MoS<sub>2<\/sub>\uff0c1.2 nm\u5c42\u95f4\u9650\u57dfNiFe@MoS<sub>2<\/sub>\u548c\u5e73\u9762NiFe@MoS<sub>2<\/sub>\u7684PDOS\u7ed3\u679c\uff0c\u5176\u4e2dd\u5e26\u4e2d\u5fc3\u4f4d\u7f6e\u7528\u7ea2\u8272\u865a\u7ebf\u6807\u8bb0\u3002<\/section>\n<section><img decoding=\"async\" title=\"3\" src=\"http:\/\/9794.seohost.cn\/storage\/9794\/article\/20230514\/1684027530783701.jpg\" alt=\"3\" \/><\/section>\n<section><strong>\u56fe3<\/strong>. \uff08a\uff09\u4e8c\u786b\u5316\u94bc\u8584\u819c\u7684HAADF-STEM\u56fe\u50cf\uff1b\uff08b\uff09\u4ece\uff08a\uff09\u4e2d\u54c1\u7ea2\u8272\u865a\u7ebf\u77e9\u5f62\u533a\u57df\u91c7\u96c6\u5f97\u5230\u7684HAADF\u5f3a\u5ea6\u5256\u9762\u56fe\uff1b\uff08c\uff09\u7528LMBE\u65b9\u6cd5\u5728\u5355\u5c42\u4e8c\u786b\u5316\u94bc\u8584\u819c\u4e0a\u951a\u5b9aNi\u548cFe 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K\u8fb9\uff08k\uff09\u7684\u5085\u91cc\u53f6\u53d8\u6362\u56fe\uff0cNi\uff08\u6216Fe\uff09\u7b94\u4e3a\u5bf9\u6bd4\u6837\uff0c\u5176\u4e2d\u63d2\u56fe\u662f\u76f8\u5bf9\u5e94\u7684XANES\u5149\u8c31\u3002<\/section>\n<section><img decoding=\"async\" title=\"4\" src=\"http:\/\/9794.seohost.cn\/storage\/9794\/article\/20230514\/1684027540561021.jpg\" alt=\"4\" \/><\/section>\n<section><strong>\u56fe4<\/strong>. \u5c42\u95f4\u9650\u57dfNiFe@MoS<sub>2<\/sub>\u5728HER\u8fc7\u7a0b\u4e2d\u7684\uff08a\uff09\u6781\u5316\u66f2\u7ebf\u548c\uff08b\uff09\u5bf9\u5e94\u7684Tafel\u56fe\uff0c\u5176\u4e2d\u5e73\u9762NiFe@MoS<sub>2<\/sub>\u3001\u5c42\u95f4\u9650\u57dfSv@MoS<sub>2<\/sub>\u548c\u73bb\u78b3\u7535\u6781\u548c20%Pt\/C\u7528\u4f5c\u5bf9\u6bd4\u6837\uff1b\uff08c\uff09\u5e73\u9762NiFe@MoS<sub>2<\/sub>\u548c\u5c42\u95f4\u9650\u57dfNiFe@MoS<sub>2<\/sub>\u7684<em>j<\/em>-t\u6d4b\u8bd5\uff1b\u5c42\u95f4\u9650\u57dfNiFe@MoS<sub>2<\/sub>\u5728OER\u8fc7\u7a0b\u4e2d\u7684\uff08d\uff09\u6781\u5316\u66f2\u7ebf\u548c\uff08e\uff09\u5bf9\u5e94\u7684Tafel\u56fe\uff0c\u5176\u4e2d\u5e73\u9762NiFe@MoS<sub>2<\/sub>\u3001\u5c42\u95f4\u9650\u57dfSv@MoS<sub>2<\/sub>\u548cIrO<sub>2<\/sub>\u7528\u4f5c\u5bf9\u6bd4\u6837\uff1b\uff08f\uff09\u5e73\u9762NiFe@MoS<sub>2<\/sub>\u548c\u5c42\u95f4\u9650\u57dfNiFe@MoS<sub>2<\/sub>\u7684<em>j<\/em>-t\u6d4b\u8bd5\u3002<\/section>\n<section><img decoding=\"async\" title=\"5\" src=\"http:\/\/9794.seohost.cn\/storage\/9794\/article\/20230514\/1684027551199218.jpg\" alt=\"5\" \/><\/section>\n<section><strong>\u56fe5<\/strong>.\uff08a\uff09\u5728\u9178\u6027\u7535\u89e3\u6db2\u4e2d\uff0c\u5c42\u95f4\u9650\u57dfNiFe@MoS<sub>2<\/sub>\u7684\u7535\u89e3\u6c34\u5b9e\u9a8c\u88c5\u7f6e\u793a\u610f\u56fe\uff1b\uff08b\uff09\u5c42\u95f4\u9650\u57dfNiFe@MoS<sub>2<\/sub>\u3001\u5e73\u9762NiFe@MoS<sub>2<\/sub>\u548c\u5c42\u95f4\u9650\u57dfSv@MoS<sub>2<\/sub>\u7684\u5168\u89e3\u6c34\u6781\u5316\u66f2\u7ebf\uff1b\uff08c\uff09\u5e73\u9762NiFe@MoS<sub>2<\/sub>\u548c\u5c42\u95f4\u9650\u57dfNiFe@MoS<sub>2<\/sub>\u768416\u5c0f\u65f6\u8ba1\u65f6\u7535\u4f4d\u6d4b\u8bd5; \uff08d\uff09\u5c42\u95f4\u9650\u57dfNiFe@MoS<sub>2\u00a0<\/sub>\u5728\u9ad8\u7535\u6d41\u5bc6\u5ea6\uff08150 mA\/cm<sup>2<\/sup>\uff09\u4e0b\u7684100\u5c0f\u65f6<em>j<\/em>-t\u6d4b\u8bd5\uff1b\uff08e\uff09\u5728<em>j<\/em>=150 mA\/cm<sup>2<\/sup>\u9ad8\u7535\u6d41\u5bc6\u5ea6\u4e0b\u8fdb\u884c100 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