{"id":47620,"date":"2023-04-06T08:32:16","date_gmt":"2023-04-06T00:32:16","guid":{"rendered":"https:\/\/www.chemhui.com\/?p=47620"},"modified":"2023-03-21T10:33:07","modified_gmt":"2023-03-21T02:33:07","slug":"acs-catalysis%ef%bc%9a%e5%89%96%e5%b9%bd%e6%9e%90%e5%be%ae%ef%bc%81%e6%8f%ad%e7%a4%bain2o3-%e9%87%91%e5%b1%9e%e7%95%8c%e9%9d%a2%e4%b8%8a%e9%ab%98%e7%94%b2%e9%86%87%e9%80%89%e6%8b%a9%e6%80%a7%e7%9a%84","status":"publish","type":"post","link":"http:\/\/www.chemhui.com\/acs-catalysis%ef%bc%9a%e5%89%96%e5%b9%bd%e6%9e%90%e5%be%ae%ef%bc%81%e6%8f%ad%e7%a4%bain2o3-%e9%87%91%e5%b1%9e%e7%95%8c%e9%9d%a2%e4%b8%8a%e9%ab%98%e7%94%b2%e9%86%87%e9%80%89%e6%8b%a9%e6%80%a7%e7%9a%84\/","title":{"rendered":"ACS Catalysis\uff1a\u5256\u5e7d\u6790\u5fae\uff01\u63ed\u793aIn2O3-\u91d1\u5c5e\u754c\u9762\u4e0a\u9ad8\u7532\u9187\u9009\u62e9\u6027\u7684\u539f\u5b50\u7ed3\u6784\u8d77\u6e90"},"content":{"rendered":"

CO2<\/sub>\u52a0\u6c22\u5236\u7532\u9187\u5177\u6709\u51cf\u5c11\u78b3\u6392\u653e\u548c\u5728\u4e00\u6b21\u53cd\u5e94\u4e2d\u751f\u4ea7\u6709\u4ef7\u503c\u7684\u5316\u5b66\u54c1\u7684\u6f5c\u529b\uff0c\u56e0\u6b64\u5176\u5177\u6709\u91cd\u8981\u7684\u73af\u5883\u548c\u7ecf\u6d4e\u610f\u4e49\u3002\u4e0e\u672a\u6539\u6027\u7684\u4f20\u7edfCu\/ZnO\/Al2<\/sub>O3<\/sub>\u50ac\u5316\u5242\u76f8\u6bd4\uff0c\u6c27\u5316\u94df\u57fa\u50ac\u5316\u5242\u7684\u7532\u9187\u9009\u62e9\u6027\u63d0\u9ad8\u4e86\u4e00\u500d(\u4ece30-50%\u63d0\u9ad8\u523060-100%)\u3002<\/p>\n

\u503c\u5f97\u6ce8\u610f\u7684\u662f\uff0c\u867d\u7136\u7532\u9187\u6536\u7387\u6709\u6240\u63d0\u9ad8\uff0c\u4f46\u662f\u5bf9\u4e8e\u5206\u6563\u5728\u6c27\u5316\u94df(M\/In2<\/sub>O3<\/sub>\uff0cM=Pd\uff0cNi\uff0cAu\u7b49)\u4e0a\u7684\u5404\u79cd\u6d3b\u6027\u91d1\u5c5e\u50ac\u5316\u5242\uff0c\u5c3d\u7ba1\u6dfb\u52a0\u7684\u91d1\u5c5e\u5177\u6709\u4e0d\u540c\u7684\u5316\u5b66\u6027\u8d28\uff0c\u5176\u9009\u62e9\u6027\u4ecd\u7136\u4e0e\u666e\u901aIn2<\/sub>O3<\/sub>\u76f8\u4f3c\u3002<\/p>\n

\"1\"<\/p>\n

\"2\"<\/p>\n

\u4e3a\u4e86\u7814\u7a76\u8fd9\u79cd\u884c\u4e3a\u80cc\u540e\u7684\u73b0\u8c61\uff0c\u5e03\u9c81\u514b\u9ed1\u6587\u56fd\u5bb6\u5b9e\u9a8c\u5ba4Ping Liu<\/strong>\u548cJos\u00e9 A. Rodriguez<\/strong>\u7b49\u4f7f\u7528RuO2<\/sub>\/In2<\/sub>O3<\/sub>\u4f5c\u4e3a\u6a21\u578b\u50ac\u5316\u5242\u6765\u7814\u7a76\u6d3b\u6027\u4e2d\u5fc3\u7684\u52a8\u6001\u6027\u8d28\u3002AP-XPS\u3001\u539f\u4f4dXAFS\u548cTR-XRD\u7ed3\u679c\u8868\u660e\uff0cRuO2<\/sub>\/In2<\/sub>O3<\/sub>\u50ac\u5316\u5242\u5728\u53cd\u5e94\u73af\u5883\u4e2d\u7684\u7ed3\u6784\u5177\u6709\u9ad8\u5ea6\u7684\u52a8\u6001\u6027\u3002<\/p>\n

\u5177\u4f53\u800c\u8a00\uff0c\u5728\u53cd\u5e94\u6761\u4ef6\u4e0b\uff0cRu\u7eb3\u7c73\u7c92\u5b50\u4fc3\u8fdb\u4e86In2<\/sub>O3<\/sub>\u7684\u8fd8\u539f\uff0c\u4ece\u800c\u4ea7\u751f\u4e86\u5177\u6709\u6c27\u7a7a\u4f4d\u7684In2<\/sub>O3-x<\/sub>\uff1b\u5728\u4e00\u5b9a\u6d53\u5ea6\u7684\u6c27\u7a7a\u4f4d\u4f5c\u7528\u4e0b\uff0cIn2<\/sub>O3-x<\/sub>\u4f1a\u8fc1\u79fb\u5230Ru\u56e2\u7c07\u8868\u9762\uff0c\u5f62\u6210\u70ed\u529b\u5b66\u9a71\u52a8\u7684\u5305\u8986\u7ed3\u6784\u3002<\/p>\n

\"3\"<\/p>\n

\"4\"<\/p>\n

\u7531RuOx<\/sub>\u548cIn2<\/sub>O3-x<\/sub>\u805a\u96c6\u4f53\u4fee\u9970\u7684Ru0<\/sup>\u7eb3\u7c73\u9897\u7c92\u7ec4\u6210\u7684\u72ec\u7279\u7684\u5305\u8986\u7ed3\u6784\uff0c\u53ef\u4ee5\u901a\u8fc7\u963b\u65adRu0<\/sup>\u4f4d\u70b9\u6765\u6291\u5236CH4<\/sub>\u7684\u5f62\u6210\uff0c\u540c\u65f6\u4ea7\u751f\u754c\u9762RuOx<\/sub>\u2212In2<\/sub>O3-x<\/sub>\u4f4d\u70b9\u53ef\u7528\u4e8eCO2<\/sub>\u9009\u62e9\u6027\u52a0\u6c22\u5236\u7532\u9187\u3002\u4e0e\u666e\u901aIn2<\/sub>O3<\/sub>\u76f8\u6bd4\uff0c\u6240\u5236\u5907\u7684\u50ac\u5316\u5242\u7684\u7532\u9187\u9009\u62e9\u6027\u753162.4%\u63d0\u9ad8\u523074.7%\uff0c\u4ea7\u7387\u75310.25\u63d0\u9ad8\u52300.59 gMeOH<\/sub>\u00a0h\u22121<\/sup>\u00a0gcat<\/sub>\u22121<\/sup>\u3002<\/p>\n

\u5bc6\u5ea6\u6cdb\u51fd\u7406\u8bba(DFT)\u8ba1\u7b97\u8868\u660e\uff0c\u5728\u6c27\u7a7a\u4f4d\u5f62\u6210\u3001CO2<\/sub>\u6d3b\u5316\u4ee5\u53ca\u8fdb\u4e00\u6b65\u8f6c\u5316\u4e3a\u7532\u9187\u7b49\u65b9\u9762\uff0cIn2<\/sub>O3-x<\/sub>\u8986\u76d6\u5c42\u6bd4\u672c\u4f53In2<\/sub>O3<\/sub>\u5177\u6709\u66f4\u9ad8\u7684\u6d3b\u6027\uff0c\u8fd9\u662f\u5bfc\u81f4\u6d3b\u6027\u589e\u5f3a\u7684\u539f\u56e0\u3002\u603b\u7684\u6765\u8bf4\uff0c\u8fd9\u9879\u5de5\u4f5c\u63ed\u793a\u4e86In2<\/sub>O3<\/sub>\u57fa\u50ac\u5316\u5242\u5bf9\u53cd\u5e94\u73af\u5883\u54cd\u5e94\u7684\u52a8\u6001\u7ed3\u6784\uff0c\u4e3a\u5408\u7406\u8bbe\u8ba1\u9009\u62e9\u6027\u5408\u6210\u7532\u9187\u7684\u6750\u6599\u63d0\u4f9b\u4e86\u6307\u5bfc\u3002<\/p>\n

Atomic Structural Origin of the High Methanol Selectivity over In2<\/sub>O3<\/sub>\u2013Metal Interfaces: Metal\u2013Support Interactions and the Formation of a InOx Overlayer in Ru\/In2<\/sub>O3<\/sub>\u00a0Catalysts during CO2<\/sub>\u00a0Hydrogenation. ACS Catalysis, 2023. DOI: 10.1021\/acscatal.2c06029<\/p>\n","protected":false},"excerpt":{"rendered":"

CO2\u52a0\u6c22\u5236\u7532\u9187\u5177\u6709\u51cf\u5c11\u78b3\u6392\u653e\u548c\u5728\u4e00\u6b21\u53cd\u5e94\u4e2d\u751f\u4ea7\u6709\u4ef7\u503c\u7684\u5316\u5b66\u54c1\u7684\u6f5c\u529b\uff0c\u56e0\u6b64\u5176\u5177\u6709\u91cd\u8981\u7684\u73af\u5883\u548c\u7ecf\u6d4e\u610f\u4e49\u3002\u4e0e\u672a\u6539\u6027 […]<\/p>\n","protected":false},"author":326,"featured_media":0,"comment_status":"open","ping_status":"open","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[14],"tags":[],"class_list":["post-47620","post","type-post","status-publish","format-standard","hentry","category-tuijianyuedu"],"_links":{"self":[{"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/posts\/47620","targetHints":{"allow":["GET"]}}],"collection":[{"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/posts"}],"about":[{"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/users\/326"}],"replies":[{"embeddable":true,"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/comments?post=47620"}],"version-history":[{"count":1,"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/posts\/47620\/revisions"}],"predecessor-version":[{"id":47621,"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/posts\/47620\/revisions\/47621"}],"wp:attachment":[{"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/media?parent=47620"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/categories?post=47620"},{"taxonomy":"post_tag","embeddable":true,"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/tags?post=47620"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}