{"id":47596,"date":"2023-04-03T09:17:44","date_gmt":"2023-04-03T01:17:44","guid":{"rendered":"https:\/\/www.chemhui.com\/?p=47596"},"modified":"2023-03-19T09:19:33","modified_gmt":"2023-03-19T01:19:33","slug":"angew-chem-%ef%bc%9a%e5%af%8c%e7%94%b5%e5%ad%90%e7%ad%96%e7%95%a5%e7%a8%b3%e5%ae%9aco2%e2%88%92%e5%ae%9e%e7%8e%b0%e9%ab%98%e6%95%88co2%e7%94%b5%e8%bf%98%e5%8e%9f","status":"publish","type":"post","link":"http:\/\/www.chemhui.com\/angew-chem-%ef%bc%9a%e5%af%8c%e7%94%b5%e5%ad%90%e7%ad%96%e7%95%a5%e7%a8%b3%e5%ae%9aco2%e2%88%92%e5%ae%9e%e7%8e%b0%e9%ab%98%e6%95%88co2%e7%94%b5%e8%bf%98%e5%8e%9f\/","title":{"rendered":"Angew. Chem. \uff1a\u5bcc\u7535\u5b50\u7b56\u7565\u7a33\u5b9aCO2\u2022\u2212\u5b9e\u73b0\u9ad8\u6548CO2\u7535\u8fd8\u539f"},"content":{"rendered":"
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\u5229\u7528\u7eff\u8272\u53ef\u6301\u7eed\u7684\u592a\u9633\u80fd\uff0c\u5c06CO2<\/sub>\u7535\u50ac\u5316\u8fd8\u539f\uff08CO2<\/sub>RR\uff09\u4e3a\u9ad8\u9644\u52a0\u503c\u7684\u7532\u9178\uff08\u76d0\uff09\u662f\u7f13\u89e3\u76ee\u524d\u5168\u7403\u6e29\u5ba4\u6548\u5e94\u548c\u80fd\u6e90\u5371\u673a\uff0c\u5b9e\u73b0\u78b3\u4e2d\u548c\u7684\u4e00\u79cd\u6709\u524d\u666f\u7684\u9014\u5f84\u3002\u7136\u800c\uff0c\u76ee\u524dCO2<\/sub>RR\u5230\u7532\u9178\u76d0\u7684\u9009\u62e9\u6027\u548c\u6d3b\u6027\u4ecd\u7136\u666e\u904d\u8f83\u4f4e\uff0c\u9002\u7528\u73af\u5883\u8303\u56f4\u8f83\u7a84\uff0c\u4e3b\u8981\u5b58\u5728\u4ee5\u4e0b\u4e24\u4e2a\u5173\u952e\u95ee\u9898\uff1a\uff081\uff09\u4f5c\u4e3aCO2<\/sub>RR\u7684\u7b2c\u4e00\u6b65\uff0c\u4eceCO2<\/sub>\u5230CO2<\/sub>\u2022\u2212<\/sup>\u81ea\u7531\u57fa\u9634\u79bb\u5b50\u7684\u76f4\u63a5\u7535\u5b50\u8f6c\u79fb\u8fc7\u7a0b\u9700\u8981\u9ad8\u8fbe\u22121.9 V (vs RHE)\u7684\u7535\u52bf\uff0c\u8fd9\u4f7f\u5f97CO2<\/sub>\u6d3b\u5316\u6210\u4e3a\u70ed\u529b\u5b66\u8fc7\u7a0b\u7684\u9650\u5236\u6b65\u9aa4\uff1b\uff082\uff09CO2<\/sub>\u5206\u5b50\u5bb9\u6613\u4e0e\u5e38\u7528\u7684\u78b1\u6027\u6216\u4e2d\u6027\u7535\u89e3\u8d28\u4e2d\u7684OH\u2212<\/sup>\u53cd\u5e94\u751f\u6210CO3<\/sub>2\u2212<\/sup>\u6216HCO3<\/sub>\u2212<\/sup>\uff0c\u8fd9\u5c31\u964d\u4f4e\u4e86CO2<\/sub>\u7684\u5229\u7528\u7387\uff0c\u751a\u81f3\u4f1a\u5835\u585e\u6c14\u4f53\u6269\u6563\u7535\u6781\uff08GDE\uff09\u4e2d\u7684CO2<\/sub>\u4f20\u8f93\u901a\u9053\u3002<\/p>\n<\/section>\n<\/section>\n<\/section>\n<\/section>\n<\/section>\n

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\u8fd1\u65e5\uff0c\u5c71\u4e1c\u5927\u5b66\u7a0b\u5408\u950b\u6559\u6388\u3001\u9ec4\u67cf\u6807\u6559\u6388\u56e2\u961f\u901a\u8fc7\u7535\u5b50\u7ed3\u6784\u8c03\u63a7\u7b56\u7565\u5236\u5907\u4e86\u4e00\u79cd\u5bcc\u7535\u5b50\u7684Bi\u7eb3\u7c73\u7247\uff08Cu-Bi\u53cc\u91d1\u5c5e\u7eb3\u7c73\u7ed3\u6784\uff09\uff0c\u5176\u4e2dCu\u4f5c\u4e3a\u7535\u5b50\u7ed9\u4f53\u5411Bi\u7535\u5b50\u53d7\u4f53\u63d0\u4f9b\u7535\u5b50\u3002\u8fd9\u79cd\u5bcc\u7535\u5b50Bi\u7eb3\u7c73\u7247\u80fd\u591f\u6709\u6548\u4fc3\u8fdbCO2<\/sub>\u7684\u6d3b\u5316\uff0c\u540c\u65f6\u5b9e\u73b0\u4e86\u5168pH\u8303\u56f4\u4e0b\u7684\u9ad8\u6548CO2<\/sub>\u7535\u50ac\u5316\u8fd8\u539f\u3002<\/p>\n<\/section>\n<\/section>\n<\/section>\n<\/section>\n<\/section>\n
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\u5728\u22120.8\u81f3\u22121.2 V vs RHE\u7684\u78b1\u6027\u7535\u89e3\u8d28\u4e2d\uff0c\u53cc\u91d1\u5c5eCu-Bi\u4e0a\u7684\u7532\u9178\u76d0\u7684\u9009\u62e9\u6027\u80fd\u591f\u4fdd\u6301>90%\uff0c\u5728\u22121.0 V vs RHE\u65f6\u6700\u5927\u503c\u7ea6\u4e3a93.2%\u3002\u540c\u6837\uff0c\u5728\u4e2d\u6027\u548c\u9178\u6027\u7535\u89e3\u8d28\u4e2d\uff0c\u7532\u9178\u76d0\u7684\u9009\u62e9\u6027\u4e5f\u53ef\u4ee5\u5206\u522b\u5728\u22120.8\u81f3\u22121.1 V vs RHE\u548c\u22121.0\u81f3\u22121.1 V vs RHE\u65f6\u4fdd\u6301\u226590%\u3002\u4e0e\u4e4b\u5f62\u6210\u9c9c\u660e\u5bf9\u6bd4\u7684\u662f\uff0c\u5bf9\u4e8eHOD-Cu\u548c\u7eafBi\uff0c\u5728\u9178\u6027\u3001\u4e2d\u6027\u548c\u78b1\u6027\u6eb6\u6db2\u4e2d\uff0c\u5728\u22121.0 V vs RHE\u65f6\u76f8\u5e94\u7684\u7532\u9178\u76d0\u7684\u9009\u62e9\u6027\u5206\u522b\u4f4e\u4e8e52%\u548c82%\u3002<\/p>\n<\/section>\n<\/section>\n<\/section>\n<\/section>\n<\/section>\n
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\u901a\u8fc7Tafel\u659c\u7387\u6d4b\u8bd5\u53d1\u73b0\uff0c\u5bcc\u7535\u5b50Bi\u7eb3\u7c73\u7247\u5728\u52a8\u529b\u5b66\u4e0a\u66f4\u6709\u4f18\u52bf\u3002CO2<\/sub>–<\/sup>\u7a0b\u5e8f\u5347\u6e29\u8131\u9644\u6d4b\u8bd5\u8bc1\u660e\u4e86CO2<\/sub>\u4e0e\u5bcc\u7535\u5b50Bi\u7eb3\u7c73\u7247\u7684\u7ed3\u5408\u66f4\u7262\u56fa\u3002\u8fdb\u4e00\u6b65\u7684\u539f\u4f4d\u7535\u5316\u5b66\u62c9\u66fc\u5149\u8c31\u7ed3\u5408\u7406\u8bba\u8ba1\u7b97\u8868\u660e\uff0c\u5bcc\u7535\u5b50Bi\u7eb3\u7c73\u7247\u80fd\u591f\u6709\u6548\u6d3b\u5316CO2<\/sub>\u5206\u5b50\uff0c\u4fc3\u8fdb\u4e86CO2<\/sub>\u2022\u2212<\/sup>\u81ea\u7531\u57fa\u9634\u79bb\u5b50\u4e2d\u95f4\u4f53\u7684\u5f62\u6210\uff0c\u4f7f\u5176\u8fdb\u4e00\u6b65\u8d28\u5b50\u5316\u5f62\u6210*OCHO\u4e2d\u95f4\u4f53\uff0c\u540c\u65f6\u80fd\u663e\u8457\u964d\u4f4eCO2<\/sub>\u8fd8\u539f\u5230HCOOH\u4ea7\u7269\u7684\u80fd\u91cf\u52bf\u5792\u3002\u8be5\u5de5\u4f5c\u63d0\u4f9b\u4e86\u4e00\u79cd\u6709\u6548\u7684\u7535\u5b50\u7ed3\u6784\u8c03\u63a7\u7b56\u7565\uff0c\u4fc3\u8fdbCO2<\/sub>\u2022\u2212<\/sup>\u81ea\u7531\u57fa\u9634\u79bb\u5b50\u7684\u5f62\u6210\uff0c\u5b9e\u73b02<\/sub>\u8fd8\u539f\u751f\u6210\u7532\u9178\u76d0\u7684\u9ad8\u6d3b\u6027\u3001\u9ad8\u9009\u62e9\u6027\u548c\u9ad8\u7a33\u5b9a\u6027\u3002\u6b64\u5916\uff0c\u8fd9\u79cd\u7535\u5b50\u7ed9\u4f53-\u53d7\u4f53\u7b56\u7565\u53ef\u4ee5\u6269\u5c55\u5230\u5176\u5b83\u50ac\u5316\u5242\uff0c\u4ee5\u671f\u5b9e\u73b0CO2<\/sub>\u8fd8\u539f\u5230\u7279\u5b9a\u4ea7\u7269\u7684\u9ad8\u6027\u80fd\u3002<\/p>\n<\/section>\n<\/section>\n<\/section>\n<\/section>\n<\/section>\n
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Electron-Rich Bi Nanosheets Promotes CO2<\/sub>\u2022\u2212<\/sup>\u00a0Formation for High-Performance and pH-Universal Electrocatalytic CO2<\/sub>\u00a0Reduction<\/p>\n

Zaiqi Li, Bin Sun, Difei Xiao, Zeyan Wang, Yuanyuan Liu, Zhaoke Zheng, Peng Wang, Ying Dai, Hefeng Cheng and Baibiao Huang<\/p>\n

Angewandte Chemie International Edition<\/em><\/p>\n

DOI:\u00a010.1002\/anie.202217569<\/p>\n<\/section>\n<\/section>\n<\/section>\n

 <\/p>\n","protected":false},"excerpt":{"rendered":"

\u5229\u7528\u7eff\u8272\u53ef\u6301\u7eed\u7684\u592a\u9633\u80fd\uff0c\u5c06CO2\u7535\u50ac\u5316\u8fd8\u539f\uff08CO2RR\uff09\u4e3a\u9ad8\u9644\u52a0\u503c\u7684\u7532\u9178\uff08\u76d0\uff09\u662f\u7f13\u89e3\u76ee\u524d\u5168\u7403\u6e29\u5ba4\u6548\u5e94\u548c\u80fd\u6e90\u5371\u673a […]<\/p>\n","protected":false},"author":326,"featured_media":0,"comment_status":"open","ping_status":"open","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[14],"tags":[],"class_list":["post-47596","post","type-post","status-publish","format-standard","hentry","category-tuijianyuedu"],"_links":{"self":[{"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/posts\/47596","targetHints":{"allow":["GET"]}}],"collection":[{"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/posts"}],"about":[{"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/users\/326"}],"replies":[{"embeddable":true,"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/comments?post=47596"}],"version-history":[{"count":1,"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/posts\/47596\/revisions"}],"predecessor-version":[{"id":47597,"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/posts\/47596\/revisions\/47597"}],"wp:attachment":[{"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/media?parent=47596"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/categories?post=47596"},{"taxonomy":"post_tag","embeddable":true,"href":"http:\/\/www.chemhui.com\/wp-json\/wp\/v2\/tags?post=47596"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}